Optimization and modeling of photocatalytic degradation of Direct Blue 71 from contaminated water by TiO2 nanoparticles: Response surface methodology approach (RSM)

Massoudinejad, Mohamadreza; Sadani, Mohsen; Gholami, Zeinab; Rahmati, Zeinab; Javaheri, Masoume; Keramati, Hassan; Sarafraz, Mansour; Avazpour, Moayed; Shiri, Sabah

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	Optimization and modeling of photocatalytic degradation of Direct Blue 71 from contaminated water by TiO2 nanoparticles: Response surface methodology approach (RSM)
Iranian Journal of Catalysis
مقاله 4، دوره 9، شماره 2، شهریور 2019، صفحه 121-132 اصل مقاله (1.67 M)
نوع مقاله: Articles
نویسندگان
Mohamadreza Massoudinejad¹؛ Mohsen Sadani¹؛ Zeinab Gholami²؛ Zeinab Rahmati³؛ Masoume Javaheri³؛ Hassan Keramati⁴؛ Mansour Sarafraz⁵؛ Moayed Avazpour^* ³؛ Sabah Shiri^* ⁶
¹School of Public Health and Safety, Shahid Beheshti University of Medical Sciences, Tehran, Iran.
²Student Research Committee, School of Public Health, Tehran University of Medical Sciences, Tehran, Iran.
³Department of Environmental Health Engineering, School of Public Health, Ilam University of Medical Science, Ilam, Iran.
⁴Department of Environmental Health Engineering, School of Public Health, Semnan University of Medical Sciences, Semnan, Iran.
⁵Student Research Committee, School of Public Health and Safety, Shahid Beheshti University of Medical Sciences, Tehran, Iran.
⁶Department of Chemistry. Payame Noor University. P.O. Box 19395-4697, Tehran, Iran.
چکیده
In the current survey, the removal of dye from contaminated water was studied by photocatalytic degradation using TiO₂ nanoparticles with respect to pH, TiO₂ dosage, reaction time, temperature and initial dye concentration. TiO₂ nanoparticles were investigated by XRD, FESEM and FT-IR.The RSM was chosen to study the composition effects of input independent factors and one dependent output response (removal efficiency). The P-value (2.2 × 10⁻¹⁶), F-value (1832), R² (multiple R-squared: 0.9985, adjusted R-squared: 0.9972), and lack of fit (0.432) indicate that the reduced full second order model is highly significant for dye removal by TiO₂ nanoparticles.The maximum percentage removal of dye, 90.2%, was achieved at optimum operating conditions including pH=6.5, TiO₂ dose (1.2 g L^-1), contact time (67.5 min), temperature ( ), and dye concentrations (55 mg L^-1)), respectively.The maximum removal efficiency was calculated to be 100%, using regression coefficients derived from the model and the Solver “Add-ins”.The results indicated that the TiO₂ photocatalyst was very proper for the removal dye from contaminated water, and it had good efficiency in eliminating textile dyes.
کلیدواژه‌ها
TiO2؛ Photocatalyst؛ Degradation؛ Direct blue 71؛ Optimization؛ RSM

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Optimization and modeling of photocatalytic degradation of Direct Blue 71 from contaminated water by TiO2 nanoparticles: Response surface methodology approach (RSM)