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Nourozi Rad, Vida, Anbia, Mansoor, Hossaini Sadr, Moayed, Zare, Karim. (1399). Catalytic performance of Ni–Cu/TiO2 catalyst for conversion of H2S and SO2 to sulfur. نشریه علمی پژوهشی دانشگاه آزاد اسلامی, 11(4), 217-222. doi: https://doi.org/10.1007/s40090-020-00217-x
Vida Nourozi Rad; Mansoor Anbia; Moayed Hossaini Sadr; Karim Zare. "Catalytic performance of Ni–Cu/TiO2 catalyst for conversion of H2S and SO2 to sulfur". نشریه علمی پژوهشی دانشگاه آزاد اسلامی, 11, 4, 1399, 217-222. doi: https://doi.org/10.1007/s40090-020-00217-x
Nourozi Rad, Vida, Anbia, Mansoor, Hossaini Sadr, Moayed, Zare, Karim. (1399). 'Catalytic performance of Ni–Cu/TiO2 catalyst for conversion of H2S and SO2 to sulfur', نشریه علمی پژوهشی دانشگاه آزاد اسلامی, 11(4), pp. 217-222. doi: https://doi.org/10.1007/s40090-020-00217-x
Nourozi Rad, Vida, Anbia, Mansoor, Hossaini Sadr, Moayed, Zare, Karim. Catalytic performance of Ni–Cu/TiO2 catalyst for conversion of H2S and SO2 to sulfur. نشریه علمی پژوهشی دانشگاه آزاد اسلامی, 1399; 11(4): 217-222. doi: https://doi.org/10.1007/s40090-020-00217-x

Catalytic performance of Ni–Cu/TiO2 catalyst for conversion of H2S and SO2 to sulfur

International Journal of Industrial Chemistry
دوره 11، شماره 4، اسفند 2020، صفحه 217-222
نوع مقاله: research article
شناسه دیجیتال (DOI): https://doi.org/10.1007/s40090-020-00217-x
نویسندگان
Vida Nourozi Rad1؛ Mansoor Anbia* 2؛ Moayed Hossaini Sadr3؛ Karim Zare1
1Department of Chemistry, Science and Research Branch, Islamic Azad University, Poonak-Hesarak, Tehran, Iran
2Research Laboratory of Nanoporous Materials, Faculty of Chemistry, Iran University of Science and Technology, Narmak, 16846-13114, Tehran, Iran
3Department of Chemistry, Faculty of Science, Azarbaijan Shahid Madani University, Tabriz, Iran
چکیده
The anatase TiO2-supported Ni–Cu bimetallic catalyst was prepared by Co-impregnation method and after shaping by three binders (bentonite, polyethylene glycol and poly vinyl alcohol) into extrudes, the effect of calcining temperature (200 °C, 400 °C, 600 °C and 800 °C) and calcining time (1, 3, 5 and 7 h) on the extrudes were investigated. According to the obtained results, the catalyst prepared at calcining temperature of 600 °C and calcining time of 5 h was selected as the optimal catalyst due to its anatase pure phase, high crystallinity and relatively high surface area. The as-prepared shape catalyst was evaluated as a Claus catalyst for conversion of H2S, CS2 and SO2 into elemental sulfur and provides high conversion of H2S 72.67%, CS2 69.77% and SO2 84.78%. The results indicated that the shaped catalyst with 75.50% of gas conversion efficiency is more active than the commercial Claus catalyst with 62.05% of conversion efficiency.
کلیدواژه‌ها
Anatase؛ Claus catalyst؛ Calcining؛ Co-impregnation؛ Elemental sulfur؛ Extrude؛ Gas conversion
آمار
تعداد مشاهده مقاله: 74


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