MgO support mediated enhancement of La2BMnO6 (B = Co, Ni) perovskite oxide in catalytic combustion of propane

Iranian Journal of Catalysis

مقاله 9، دوره 13، شماره 2، شهریور 2023، صفحه 211-222   

نوع مقاله: Articles

شناسه دیجیتال (DOI): 10.30495/ijc.2023.1984280.2004

نویسندگان

Hamidreza Roozbahani؛ Sarah Maghsoodi^* ؛ Behrouz Raei؛ Amirhossein Shahbazi Kootenaei؛ Zoha Azizi

Department of Chemical Engineering, Mahshahr Branch, Islamic Azad University, Mahshahr, Iran.

چکیده

Perovskite oxides possessing high stability and composition adjustability are effective in many applications. The La₂BMnO₆ (B=Co, Ni) double perovskite oxides were synthesized using the sol-gel method and deposited on MgO support (loading = 10, 20, and 30 wt. %) using a mechanical mixing method by an ultrasonic device. The elaborated samples were investigated for application in propane deep oxidation. The catalytic performance of these catalysts was analyzed by a variety of characterization techniques such as XRD, SEM, FTIR, TEM, and H₂-TPR. Ni-containing catalysts were found to have superior catalytic activity than the sample containing Co. The lowest catalytic activity belonged to the cobalt-containing double perovskite with 10 wt.% loading on MgO support, while the highest conversion was related to the 20La₂NiMnO₆/MgO composite oxide with T₉₀ = 434 °C. The support showed a positive impact on the performance of the catalysts. Deposition of a certain amount of perovskite oxides on the support boosted the specific surface area of the catalyst and, therefore, combined with improved reducibility, improved propane catalytic degradation.

کلیدواژه‌ها

Double perovskite oxide؛ Support؛ Composite oxide؛ Catalytic combustion؛ Propane

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